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炭气凝胶三维电极催化氧化处理苯酚废水的研究
引用本文:吕贵芬,吴丁财,符若文. 炭气凝胶三维电极催化氧化处理苯酚废水的研究[J]. 中山大学学报(自然科学版), 2008, 47(3): 75-78
作者姓名:吕贵芬  吴丁财  符若文
作者单位:1. 中山大学化学与化学工程学院,广东,广州,510275
2. 中山大学教育部聚合物复合材料及功能材料重点实验室,广东,广州,510275
基金项目:国家自然科学基金 , 广东省广州市科技基金
摘    要: 将自制的炭气凝胶用作三维电极装置的粒子电极并处理模拟苯酚废水,研究了压缩空气流速、进水pH值、溶液初始浓度及固液比等各种因素对处理结果的影响,发现:炭气凝胶三维电极对苯酚有很好的催化氧化去除效果,去除率最高可达97.5%,浓度可低至4 mg/L,循环50次后,COD去除率仍在80%以上。

关 键 词:三维电极  炭气凝胶  粒子电极  苯酚
收稿时间:2007-10-12;

Carbon Aerogels Particle Electrodes for Treatment of the Aqueous Phase Electro-catalytic Oxidation of Simulated Phenol Wastewaters
Lü Gui-fen,WU Ding-cai,FU Ruo-wen. Carbon Aerogels Particle Electrodes for Treatment of the Aqueous Phase Electro-catalytic Oxidation of Simulated Phenol Wastewaters[J]. Acta Scientiarum Naturalium Universitatis Sunyatseni, 2008, 47(3): 75-78
Authors:Lü Gui-fen  WU Ding-cai  FU Ruo-wen
Affiliation:(Materials Science Institute, PCFM Laboratory,School of Chemistry andChemical Engineering, Sun Yat sen University, Guangzhou 510275, China)
Abstract:The feasibility of using carbon aerogels (CAs) as bed electrodes in a three dimensional electrode reactor for the electrochemical treatment was studied. It was found that the removal efficiency depended on the airflow, pH, the feed phenol concentration and the ratio of aerogels mass to solution volume. Compared with commercial carbon particle electrodes, the electrodes prepared by CAs exhibited stronger activity to remove phenol simulated wastewater. 97.5% of the initial phenol can be removed after treatment for 20 min, the concentration is as low as 4 mg/L. Moreover, removal efficiency can be kept basically as high as 80% after being reused 50 times.
Keywords:three dimensional electrode  carbon aerogels  phenol  particle electrode
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