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1.
NO and N2O fluxes from agricultural soils in Beijing area   总被引:2,自引:0,他引:2  
Chinese agriculture represents one of the most intensively managed agroecosystems in the world. Typical nitrogen fertilization rates are more than three times those of the world' s average, resulting in dramatically accelerated nitrogen cycling in China. In this study, we have examined NO and N2O exchange in the upland agricultural systems of Beijing area. Inorganic and organic fertilizer treatments were arranged in order to evaluate their impact on the magnitude and proportion of trace gas emissions. Increasing inorganic fertilization rates showed a highly significant impact upon emissions of both NO and N2O. Organic matter amendment did not have a statistically significant impact on the N-gas fluxes examined here. Overall losses of added nitrogen by NO and N2O emission averaged 1.24% and 0.22% respectively over the range of treatments in this study. Results from our field study indicate that compared with other studies done elsewhere, emissions of reactive nitrogen from agricultural systems in Beijing area are not so large as expected before.  相似文献   

2.
Estimation of emissions from field burning of crop straw in China   总被引:10,自引:0,他引:10  
Emissions resulting from crop straw field burning in China, which have caused serious environmental problems in China, are estimated in this paper. From the county-level data of crop production in 2000-2003 from the government statistics, taking into account the ratio of residue and grain, the total amount of crop straw production is estimated to be about 600 Tg per year, 76% of which are rice, wheat and corn straw. With reference to the data of living standards, the percentage of crop straw burnt in fields for counties are obtained and consequently the total amount of burnt straws is approximately 140 Tg/year. With the emission factors from literature and experiments, appropriate emission factors have been obtained. The total amounts of PM, SO2, NOx3, NH3, CH4, BC, OC, VOC, CO, CO2 emissions from field burning of crop straw in China are estimated. All emissions are presented at county level. Some pollutants, such as BC, VOC, OC, CO and CO2, are contributing a major portion to the total emissions of China. This paper uses a map with resolution of 0.2°×0.2°to present the PM emissions distribution from crop straw burnt in 2003. The results show a significant regional unevenness of emissions, with larger amounts of pollutions coming from the provinces in eastern and northeast China. The regions with higher emissions per unit area are located as a belt stretching from northeast China to eastern China.  相似文献   

3.
1-Chloro-1,1-difluoroethane(HCFC-142b)was both ozone depleting substance under restriction of the Montreal Protocol on Substances that Deplete the Ozone Layer(Montreal Protocol)and potent greenhouse gas with high GWP.Controlling its emissions in China will contribute to both mitigating climate change and protecting ozone.A national emission inventory of HCFC-142b for China during 2000–2012 was established and projected to2050 based on the 2006 IPCC Guidelines for National Greenhouse Gas Inventories and the Montreal Protocol,showing that(i)in contrast to the downward trend revealed by existing researches,HCFC-142b emissions kept increasing from 0.1 kt/y in 2000 to the peak of 14.4 kt/y in2012,making China a crucial contributor to global HCFC-142b emissions and(ii)for future emission projections,a continuous increase from 14.9 kt/y in 2013 to 97.2 kt/y in2050 was anticipated under the business-as-usual(BAU)scenarios,while a reduction of about 90%of the projected BAU emissions would be obtained by fulfilling the Montreal Protocol,namely an accumulative mitigation of 1578kt HCFC-142b from 2013 to 2050,equal to 103 kt ODP and 3504 Tg CO2emissions.Emissions from each province in 2012 were also estimated to identify key emission areas.Among the 31 mainland provinces in China(Hong Kong,Macao,and Taiwan were not included),Jiangsu,Zhejiang,Shandong,and Guangdong had the highest emission ratesin 2012(2.06,1.85,1.52,and 1.04 kt/y,respectively);Zhejiang,Jiangsu,and Shanghai exhibit the strongest emission strength(0.83,0.59,and 0.54 t/km2,respectively),much higher than the average national level of 0.33t/km2.  相似文献   

4.
Emission inventories of primary particles and pollutant gases for China   总被引:12,自引:0,他引:12  
Detailed high-resolution emission inventories of primary particles(PM2.5,BC and OC) and pollutant gases(SO2,NOx,NH3,CO and VOCs) for China in 2007 were constructed on the basis of the latest fuel consumption data,mostly at the county level,and from socio-economic statistics and data on fossil and biomass fuels obtained from government agencies.New emission factors reflecting local features were also used.The calculated emissions were 13.212 Mt PM2.5,1.4 Mt BC,2.946 Mt OC,31.584 Mt SO2,23.248 Mt NOx,16.017 Mt NH3,164.856 Mt CO and 35.464 Mt VOCs.The national and regional emissions were gridded with 0.5°× 0.5° resolution for use in air quality models.Larger emissions were found in eastern and central China than in western China.The emissions estimated here are roughly equal to those obtained in previous studies,but with different contributions from because of seasonal changes in residential heating and biomass combustion.Finally,uncertainties in inventories were analyzed.  相似文献   

5.
The genetic diversity of three geographic populations of Phytophthora sojae from China and the United States was determined using random amplified polymorphic DNA (RAPD). The purpose was to explore genetic relationships among Chinese and American isolates of the organism. 21 random primers were selected among 200 random primers screened. A total of 223 reproducible RAPD fragments were scored among 111 individuals, of which 199 (89.23%) were polymorphic. Analysis of genetic variation showed that there existed higher genetic variation in the United States population in comparison to the Chinese populations. Nei's genetic identity and principal component analysis indicated that the populations of Fujian and United States are closer to each other than to Heilongjiang populations. Shannon-Wiener diversity index revealed that the United States populations have a higher genetic di- versity than that of Chinese populations. These data are in support of the hypothesis that P. sojae in the United States might not have been introduced from China.  相似文献   

6.
To account for the effects of both chemistry and flow turbulence, the present study proposes an integrated NO sub-model that combines the extended Zel’dovich mechanism and engine CFD computations to simulate the NO histories in a diesel engine. NOx sub-model parameters and pollutant formation mechanisms can be more easily investigated by solving the NOx sub-model. The new NO formation model incorporating the effects of both chemical kinetics and turbulent mixing was applied to simulate a diesel engine with a quiescent combustion chamber, and one with a re-entrant combustion chamber; the premise of the model being the reaction rate is mainly determined by a kinetic timescale and a turbulent timescale. The results indicate that the predicted NO formulation from the new model agrees well with the measured data. As the utilization of fossil fuels continues to increase, the control of NOx emissions is a worldwide concern; and it is imperative to understand fully the NOx reaction processes in combustion systems. This technology has the potential to enhance the application of various combustion techniques used to reduce NOx emissions from practical combustion systems.  相似文献   

7.
Strong pollution emissions from large urban and industrial centres in eastern China are thought to greatly impact regional air quality and global atmospheric chemistry.In this study,we investigate extensive pollution plumes over North China,observed by aircraft during the IPAC-NC(Influence of Pollution on Aerosols and Cloud Microphysics in North China)field campaign in spring 2006.Several pollution plumes were encountered,characterized by sharp and strong increases of SO2and NOx(NO plus NO2)as well as remarkable O3variability.During a flight performed downwind of the megacity Tianjin on 9 April,O3was found to be depleted at NOx>15 ppbv and enhanced at NOx mixing ratios of 6–7 ppbv.Our analysis indicates that the plumes had recently been released by industrial plants,and partly mixed with urban emissions,giving rise to the large-scale transport of air pollution and substantial degradation of air quality.  相似文献   

8.
To account for the effects of both chemistry and flow turbulence, the present study proposes an integrated NO sub-model that combines the extended Zel'dovich mechanism and engine CFD computations to simulate the NO histories in a diesel engine. NOx sub-model parameters and pollutant formation mechanisms can be more easily investigated by solving the NOx sub-model. The new NO formation model incorporating the effects of both chemical kinetics and turbulent mixing was applied to simulate a diesel engine with a quiescent combustion chamber, and one with a re-entrant combustion chamber; the premise of the model being the reaction rate is mainly determined by a kinetic timescale and a turbulent timescale. The results indicate that the predicted NO formulation from the new model agrees well with the measured data. As the utilization of fossil fuels continues to increase, the control of NOx emissions is a worldwide concern; and it is imperative to understand fully the NOx reaction processes in combustion systems. This technology has the potential to enhance the application of various combustion techniques used to reduce NOx emissions from practical combustion systems.  相似文献   

9.
This study evaluates trends in quality of nanotechnology and nanoscience papers produced by authors from the People's Republic of China (PRC). The metric used to gauge quality is ratio of highly cited nanotechnology papers to total nanotechnology papers produced in sequential time frames. The USA is both the most prolific nanotechnology publishing country and most represented country on highly cited nanotechnology papers (both in absolute numbers of highly cited papers and highly cited papers relative to total publications) over the 1998-2003 time frame, based on the SCl/SSCl databases. Some of the smaller hi-tech countries have relatively high ratios (-2) of highly cited papers to total publications (e.g. Denmark, Netherlands, Switzerland). Countries that have exhibited rapid growth in SCl/SSCl nanotechnology paper production in recent years (e.g. PRC, South Korea) had ratios an order of magnitude less than that of the USA for 1998, but by 2003 had increased to about 20% that of the USA (-2.5). PRC and South Korea have climbed in the publications rankings from 6th and 9th in 1998, respectively, to 2nd and 6th in 2005, respectively. PRC's ratio monotonically increased from 0.16 to 0.45 over the 1998-2003 period, and South Korea's ratio increased from 0.11 to about 0.6 over that same period, indicating their papers are getting more and more citations proportionately. Thus, under rapid growth conditions, PRC and South Korea have been able to increase their share of participation in highly cited papers. As of 2003, PRC and South Korea have ratios comparable to nations like Japan, France, Italy, and Australia but not yet approaching those of the highly cited countries. None of the top ten publications producing institutions are from the USA, while all of the top ten highly cited publications producers are from the USA. Over the 1998-2003 time period, the top six total publications producing institutions (globally) remained the same, with Chinese Academy of Sciences (which consists  相似文献   

10.
China’s COMPASS satellite navigation system consists of five or more geostationary (GEO) satellites.The roles of GEO satellites are to improve the regional user’s positioning accuracy and provide the continuous Radio Determination Satellite Service.The motion of GEO satellites relative to a ground tracking station is almost fixed,and regular orbit maneuvers are necessary to maintain the satellites’ allocated positions above the equator.These features present difficulties in precise orbit determination (POD).C-band ranging via onboard transponders and the L-band pseudo-ranging technique have been used in the COMPASS system.This paper introduces VLBI tracking,which has been successfully employed in the Chinese lunar exploration programs Chang’E-1 and Chang’E-2,to the POD of GEO satellites.In contrast to ranging,which measures distances between a GEO satellite and an observer,VLBI is an angular measurement technique that constrains the satellite’s position errors perpendicular to the satellite-to-observer direction.As a demonstration,the Chinese VLBI Network organized a tracking and orbit-determination experiment for a GEO navigation satellite lasting 24 h.This paper uses the VLBI delay and delay-rate data,in combination with C-band ranging data,to determine the GEO satellite’s orbit.The accuracies of the VLBI delay and delay rate data are about 3.6 ns and 0.4 ps/s,respectively.Data analysis shows that the VLBI data are able to calibrate systematic errors of the C-band ranging data,and the combination of the two observations improves orbit prediction accuracy with short-arc data,which is important for orbital recovery after maneuvers of GEO satellites.With the implementation of VLBI2010,it is possible for VLBI to be applied in the COMPASS satellite navigation system.  相似文献   

11.
In this study, mitochondrial DNA (mtDNA) analysis was carried out on 9 Bronze Age horses recovered from Dashanqian and Jinggouzi archaeological sites in Chifeng region, Inner Mongolia. China to explore the origin of Chinese domestic horses. Both mtDNA 16S rRNA gene and control region (D-loop) fragments of ancient horses were amplified and sequenced. The analysis of the highly conservative 16S rRNA gene sequences indicated that the burial environment of Chifeng region is suitable for the preservation of ancient DNA (aDNA). Combing 465 mtDNA D-loop sequences representing different breeds from East Asia, Central Asia, Near East and Europe, we constructed a phylogenetic network to investigate the relationship between ancient and modern horses. The phylogenetic network showed that the 9 horses were distributed into different modern horse clusters which were closely related to them representing a certain geographical distribution. Our results showed that the maternal genetic line of the ancient horses in Chifeng region was highly diversified, which contributed to the gene pool of modern domestic horses and suggested a complex origin of domestic horses in China.  相似文献   

12.
In this study, mitochondrial DNA (mtDNA) analysis was carried out on 9 Bronze Age horses recovered from Dashanqian and Jinggouzi archaeological sites in Chifeng region, Inner Mongolia. China to explore the origin of Chinese domestic horses. Both mtDNA 16S rRNA gene and control region (D-loop) fragments of ancient horses were amplified and sequenced. The analysis of the highly conservative 16S rRNA gene sequences indicated that the burial environment of Chifeng region is suitable for the preservation of ancient DNA (aDNA). Combing 465 mtDNA D-loop sequences representing different breeds from East Asia, Central Asia, Near East and Europe, we constructed a phylogenetic network to investigate the relationship between ancient and modern horses. The phylogenetic network showed that the 9 horses were distributed into different modern horse clusters which were closely related to them representing a certain geographical distribution. Our results showed that the maternal genetic line of the ancient horses in Chifeng region was highly diversified, which contributed to the gene pool of modern domestic horses and suggested a complex origin of domestic horses in China.  相似文献   

13.
Removal of NOx(DeNOx, NOx is the total of NO and NO2) from flue gas by radical injection has been investigated .the discharge characteristics were examined and the steady streamer corona was acquired hy adjusting the nozzle gases properly. It was Found that an increase in the voltage resulted in a decrease in the NO concentration and the concentration of the NO2 increased at tow voltages but decreased as the voltage rose to a certain level. The DeNOx efficiency increased as the applied voltage rose and reached a maximum of 70% when the voltage approached the breakdown voltage. The hypothetical mechanism of NOx removal suggested that the radicals formed in the discharge process converted the NO and NO2 into acidic species. The Monte Carlo method was used to calculate the rate coefficients and the productivity of the radicals, and then the concentrations of both NO and NO2 and the DeNOx effielencies were calculated with chemical kinetics. The calculated DeNOx efficiencies were coalparable with the experimental DeNOx efficiencies at low voltages, but were lower at high voltages.  相似文献   

14.
This study evaluates trends in quality of nanotechnology and nanoscience papers produced by au- thors from the People’s Republic of China (PRC). The metric used to gauge quality is ratio of highly cited nanotechnology papers to total nanotechnology papers produced in sequential time frames. The USA is both the most prolific nanotechnology publishing country and most represented country on highly cited nanotechnology papers (both in absolute numbers of highly cited papers and highly cited papers relative to total publications) over the 1998―2003 time frame, based on the SCI/SSCI databases. Some of the smaller hi-tech countries have relatively high ratios (~2) of highly cited papers to total publications (e.g. Denmark, Netherlands, Switzerland). Countries that have exhibited rapid growth in SCI/SSCI nanotechnology paper production in recent years (e.g. PRC, South Korea) had ratios an order of magnitude less than that of the USA for 1998, but by 2003 had increased to about 20% that of the USA (~2.5). PRC and South Korea have climbed in the publications rankings from 6th and 9th in 1998, re- spectively, to 2nd and 6th in 2005, respectively. PRC’s ratio monotonically increased from 0.16 to 0.45 over the 1998―2003 period, and South Korea’s ratio increased from 0.11 to about 0.6 over that same period, indicating their papers are getting more and more citations proportionately. Thus, under rapid growth conditions, PRC and South Korea have been able to increase their share of participation in highly cited papers. As of 2003, PRC and South Korea have ratios comparable to nations like Japan, France, Italy, and Australia but not yet approaching those of the highly cited countries. None of the top ten publications producing institutions are from the USA, while all of the top ten highly cited publica- tions producers are from the USA. Over the 1998―2003 time period, the top six total publications pro- ducing institutions (globally) remained the same, with Chinese Academy of Sciences (which consists of many research institutes) wresting the lead from Russian Academy of Sciences in 1999, and thereafter increasing the gap. Over this same time period, the USA institutions constituted about 90% of the top ten most cited papers list. For Chinese institutions specifically in the period 1998―2003, the nanotech- nology publication leading Chinese Academy of Sciences has maintained an average of about 30% of nanotechnology publications over that time frame. The second tier (in terms of quantity) for the last few years has consisted of Tsinghua University, Nanjing University, University of Science and Technology of China, Peking University, Jilin University, Zhejiang University, Shandong University, and Fudan University. Hong Kong institutions have, on average, been strong in ratio, especially City University Hong Kong, and Hong Kong University of Science and Technology, indicating significant citations.  相似文献   

15.
Degradation in visibility occurs extensively across China,creating the urgent need to better understand visibility patterns and characteristics in China.Using daily observation data from the U.S.National Climatic Data Center(NCDC)during 1976–2010,the spatial distribution and temporal trends of visibility in China,as well as seasonal and regional characteristics,were determined.The distribution of visibility was characterized by a longitudinal gradient between west and east China.The northwest of China generally experienced consistent high visibility of[20 km,while central and eastern China experienced visibility degradation and increase in haziness.The 133stations with significant downward trends in visibility were clustered around central-east China and the average reduction rate was-1.65 km/decade(from 18.5 km).The96 stations with increasing trends of visibility were mostly on the Qinghai–Tibet Plateau and Xinjiang and were closely related to a reduction in local sand storms.The average visibility in 12 key regions in China varied between9.9–17.8 km(except for 23.9 km in Urumqi),which was lower than the national average of 18.7 km.The Taiyuan–Hohhot,Guanzhong,Yangtze River Delta,Pearl River Delta and Fuzhou–Xiamen areas all encountered significant decreases in visibility,while minor increases were observed in Beijing–Tianjin–Hebei and the Cheng-Yu region.At most stations,the worst visibility was measured in winter,but the season with best visibility varied between regions.A comparison of visibility trends with the emission trends of various pollutants revealed that SO2emissions dominated the visibility degradation in eastern Chinawith NOxand volatile organic compounds playing ascending roles during the 2000s.  相似文献   

16.
Nitryl chloride (C1NO2) is a product of noc- turnal halogen activation of nitrogen oxides and has potential to impact atmospheric photochemistry. Here we report the first observation result of C1NO2 in an Asian environment. The measurements were made with a thermal decomposition chemical ionization mass spectrometer at a coastal site in southern China during late summer of 2012. A clear diurnal pattern of CINO2 was observed with nighttime 1-min average mixing ratio up to 1997 pptv, which is among the highest values ever reported in the world. The elevated CINO2 mixing ratios were observed in plumes from Hong Kong and the Pearl River Delta region compared to the lower levels in maritime air. Calculations suggest that the production of chlorine atom from photol- ysis of C1NO2 in the early morning exceeds the production of hydroxyl radical via ozone photolysis by several factors. Therefore, C1NO2 plays an important role in jump-starting the atmospheric photochemistry in polluted marine boundary layer of southern China.  相似文献   

17.
Great efforts have been made to resolve the serious environmental pollution and inevitable declining of energy resources. A review of Chinese fuel reserves and engine technology showed that compressed natural gas (CNG)/diesel dual fuel engine (DFE) was one of the best solutions for the above problems at present. In order to study and improve the emission performance of CNG/diesel DFE, an emission model for DFE based on radial basis function (RBF) neural network was developed which was a black-box input-output training data model not require priori knowledge. The RBF centers and the connected weights could be selected automatically according to the distribution of the training data in input-output space and the given approximating error. Studies showed that the predicted results accorded well with the experimental data over a large range of operating conditions from low load to high load. The developed emissions model based on the RBF neural network could be used to successfully predict and optimize the emissions performance of DFE. And the effect of the DFE main performance parameters, such as rotation speed, load, pilot quantity and injection timing, were also predicted by means of this model. In resum6, an emission prediction model for CNG/diesel DFE based on RBF neural network was built for analyzing the effect of the main performance parameters on the CO, NOx emissions of DFE. The predicted results agreed quite well with the traditional emissions model, which indicated that the model had certain application value, although it still has some limitations, because of its high dependence on the quantity of the experimental sample data.  相似文献   

18.
This study is a systematic analysis of the magnetic characteristics and heavy metal elements in soil samples collected from Lanzhou City,China.The 117 surface soil samples were measured to study the feasibility and effectiveness of environmental magnetism for evaluating heavy metal pollution in urban soils.Results of the study indicate that low-coercivity magnetite dominates the magnetic properties in the samples.The high values of the soil magnetic mineral concentration parameters and low values of magnetic particle size parameters are distributed throughout the northern area of Xigu District,the industrial zones of the eastern section of Chengguan District and the districts of the narrow sections connecting Chengguan District and the other three districts;these parameters are fundamentally consistent with the distribution of the high values of the Pollution Load Index and Nemerow Pollution Index.Semi-quantitative studies which use the environmental magnetic method to monitor pollution of heavy metals(such as As,Cr,Cu,Ni,Pb,Zn,and Fe) have shown that when xlf≤35×10-8 m 3 kg-1,it is unpolluted;when 35≤xlf <150×10-8 m3 kg-1,it is moderately polluted to unpolluted;when 150≤xlf <365×10-8 m 3 kg-1,it is moderately polluted;when 365≤xlf <750×10-8 m3 kg-1,fd %<2.7 and ARM /SIRM<0.2×10-3m A-1,it is moderately to highly polluted;when xlf ≥750×10-8 m3 kg-1,xfd %<2.7 and xARM/SIRM<0.2×10-3m A-1,it is highly polluted.The region of moderately to highly polluted distribution is caused by industry and vehicles,showing that the change of pollution in Lanzhou City bears the trend of "vehicle emission + industrial".  相似文献   

19.
Using the definition of vulnerability provided by the Intergovernmental Panel on Climate Change,this paper assesses the vulnerability of areas affected by Chinese cryospheric changes from 2001 to 2020 and from 2001 to 2050 in A1 and B1scenarios.Seven indices are used in the vulnerability assessment:glacial area fraction,interannual variability of permafrost depth,interannual variability of surface snow area fraction,interannual variability of surface runoff,interannual variability of surface temperature,interannual variability of vegetation growth,and interannual variability of the human development index.Assessment results show that the overall vulnerability of the studied areas in China increases from east to west.The areas in the middle and eastern parts of China are less vulnerable compared with western parts and parts of the Tibetan Plateau.The highest vulnerability values are found from 1981 to 2000,and the least ones are found from 2001 to 2050.The vulnerable areas increase from the period of 1981 to 2000 to the period of 2001 to 2050,and the less vulnerable areas decrease.The highly vulnerable areas increase from the period of 1981 to 2000 to the period of 2001 to 2020 and then decrease from the period of 2001 to 2020 to the period of 2001 to 2050.This decrease in vulnerability is attributed to the decrease in exposure and sensitivity to Chinese cryospheric changes along with a concomitant increase in adaptation.  相似文献   

20.
China's sizeable and uncertain carbon sink: a perspective from GOSAT   总被引:1,自引:0,他引:1  
Despite the agreement that China’s terrestrial ecosystems can provide a carbon sink and offset carbon dioxide(CO2)emissions from fossil fuels,the magnitude and spatial distribution of the sink remain uncertain.Accurate quantification of the carbon sequestration capacity of China’s terrestrial ecosystems has profound scientific and policy implications.Here,we report on the magnitude and patterns of China’s terrestrial carbon sink using the global monthly CO2flux data product from the Greenhouse gases Observing SATellite(GOSAT),the world’s first satellite dedicated to global greenhouse gas observation.We use the first year’s data from GOSAT(June 2009–May2010)that are currently available to assess China’s biospheric carbon fluxes.Our results show that China’s terrestrial ecosystems provide a carbon sink of-0.21 Pg C a-1.The consumption of fossil fuels in China leads to carbon dioxide emissions of 1.90 Pg C a-1into the atmosphere,approximately 11.1%of which is offset by China’s terrestrial ecosystems.China’s terrestrial ecosystems play a significant role in offsetting fossil fuel emissions and slowing down the buildup of CO2in the atmosphere.Our analysis based on GOSAT data offers a new perspective on the magnitude and distribution of China’s carbon sink.Our results show that China’s terrestrial ecosystems provide a sizeable and uncertain carbon sink,and further research is needed to reduce the uncertainty in its magnitude and distribution.  相似文献   

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