Pulse width effect on the dissociation probability of CH4^＋ in the intense femtosecond laser field

The electric field strength of the intense ultrashort laser pulse can reach or exceed 108 V/cm, the intensity of the Coulomb field responsible for the stability of molecules. Exposed to such intense laser fields, mole- cules become unstable, undergoing di…     

单脉冲激光热弹超声脉冲特性理论研究

对梯形激光脉冲入射到半无限弱吸收媒质中热弹激发的超声应力脉冲进行了理论研究,给出了媒质表面束缚和自由两种情况下的超声应力脉冲表达式及其理论曲线.分析表明,表面束缚时应力脉冲为单极性,表面自由时为双极性;应力脉冲比激光脉冲宽,其特性受激光脉冲形状的影响.     

Dissociation of methanol in intense femtosecond laser field

Methanol was irradiated by 80 fs laser pulse, intensity range of 10¹³–10¹⁴ W/cm². A TOF-mass spectrometer was coupled to the laser system and used to detect the ions produced. The parent ions CH₃OH⁺ appeared firstly at the laser intensity of 1.4×10¹³ W/cm². While the laser intensity was gradually increased, the parent ions were dissociated and the primary ions CH₂OH⁺ were given as verified from the irradiation of deuterated methanol (CH₃OD) showing the C—H bond cracking firstly. While the laser intensity was further increased to 2.0 × 10¹³ W/cm², the C—O bonds of the parent ions also broke to give CH₃ ⁺. When the laser intensity was higher, smaller fragment ions like CH⁺, C⁺, OH⁺ and O⁺ also appeared. Among the fragment ions, only H⁺ ion yield had anisotropic angular distribution dependence on the laser polarization vector in the dissociation of methanol. All the experimental observations show that the dissociation of methanol proceeds through stepwise mechanism but not Coulomb explosion.     

The evolution of molecular wave packet in superstrong laser fields

Summary In this note wc numerically simulate the wave packet evolution of H₂ ⁺ in superstrong laser fields with the multiple electronic-states model. The result is that the evolution process of H₂ ⁺ wave packet is mainly determined by the laser frequency. For the high-frequency fields H₂ ⁺ wave packet extends out of the interaction region step by step. However, the H₂ ⁺ wave packet is quickly dissociated in low-frequency fields. In addition, the molecular stabilization effect can be characterized at the intensity of 8 × 10¹⁵ W/cm² for the low-frequency field ω₁.     

非线性介质中超短激光脉冲的传播

系统评述了近几年有关超短脉冲传播理论及实验研究成果．针对超短脉冲在非线性介质中传播的加宽失真现象,探讨了非线性介质中超短激光脉冲传播存在的问题及其研究现状与发展趋势．     

脉冲激光加热材料的温度场解析

对脉冲激光加热解析模型进行了修正，研究了对流换热和热辐射对样品温升场分布的影响；还对表面加热模型和体加热模型进行了比较，为研究材料热学特性提供了精确的理论依据．     

Ionization and dissociation of acetonitrile by intense femtosecond laser pulse

Photoionization and photodissociation of CH3CN were studied by a linear time of flight mass spectrometer coupled with 800 nm, 50 fs laser pulses at intensities of 6.3×1013-1.2×1014 W/cm2. The laser power dependences for principal ions CH3CN+, CH2CN+, CHCN+ and CCN+ were measured, which are consistent with the numbers of photons required to produce the ions via multiphoton ionization and dissociation. The results show that eight-photon non-resonant multiphoton ionization is the main photoionization mechanism of the parent ion CH3CN+, while the fragment ions were produced through the dissociation of the molecules in the super-excited states.     

脉冲激光加热下材料的温度场研究

通过改变多种参数对单脉冲激光加热下材料温度场进行研究.     

激光短脉冲的高导数引力场

引入Teyssandier规律条件,求得线性高导数引力场方程的一般非静态解,利用高导数引入理论研究沿光波导传输的激光短脉冲产生的引力场,并与广义相对论的结果进行比较。     

强激光场中模型氢原子高次谐波的特性研究

通过数值计算求解含时的薛定谔方程,研究了单个激光脉冲作用下4个不同势函数对应的一维模型氢原子产生的高次谐波,并将其与三维真实氢原子的高次谐波比较。结果表明:势函数势阱的形状对一维模型氢原子的高次谐波强度产生较大影响,但是谐波的截止位置不变。     

强啁啾超短激光脉冲实现粒子布居的调控

采用光与物质相互作用的半经典理论方案,建立了含啁啾相位项的修正光学 Bloch 方程,并采用高精度的、快速和可靠的、修正的四阶龙格-库塔法数值求解了该方程。通过数值计算,研究了强啁啾超短激光脉冲与二能级体系的相互作用。研究结果表明,啁啾量、入射脉冲面积、脉冲宽度、失谐量都对粒子布居产生明显的调制作用,论文还研究了激光脉冲各参数对粒子布居的调控规律,由此可以通过调节强啁啾超短激光脉冲的各参数来实现对粒子布居的调控。     

Monitor and control of neuronal activities with femtosecond pulse laser

Combined with the fluorescence labeling technique, two-photon microscopy excited with femtosecond pulse laser has become an important tool for neuroscience research. In this research, the calcium signals from neurons in rat cortex slice were monitored by a custom-built two-photon microscopy, and the spontaneous calcium signals and the pharmacological responses as well as the responses to femtosecond pulse laser stimulation were recorded. The results showed that the amplitude of the cal- cium signals increased in direct proportion to the corresponding electrical activities. Glutamate induced a calcium transient, but continuous application resulted in smaller response. Simultaneous monitoring of neuronal populations distinguished the neurons of different microcircuits. The femtosecond pulse laser induced local or global calcium signals in the pyramidal neurons. The approach of interrogation and control of neural activities using femtosecond pulse laser is non-contact, nondestructive, repeatable, and without any additional substrates, which will contribute to the development of neuroscience.     

靶衬间距对脉冲激光沉积薄膜均匀性的影响

以国产脉冲激光沉积设备(PLD-Ⅲ型)在玻璃衬底上沉积Ti O2薄膜为例,研究了PLD法制膜过程中靶衬间距对薄膜均匀性的影响.实验过程中,以Ti O2陶瓷片作为靶材,玻璃作为衬底,保持其他工艺条件(如单脉冲能量、脉冲频率、沉积脉冲总数、衬底温度等)不变,专门考察了不同靶衬间距下,Ti O2薄膜在整个衬底台平面区域的沉积分布状况.结果表明,按样品的表观灰度划分,薄膜沉积的相对均匀区可分为2～3个轴对称区域,分别对应不同的沉积速率和厚度;在一定范围内调节靶衬间距(3.00～7.00 cm),可使高速率沉积区逐渐由轴对称的圆环状变为中心大圆斑(直径约2.20 cm).结合PLD沉积原理与靶衬之间的几何关系,分析了导致上述结果的机理.     

强吸收固体中激光超声脉冲的特性研究

 对梯形激光脉冲入射到半无限强吸收固体媒质中热弹激发的超声应力脉冲进行了研究.给出了媒质表面束缚和自由2种情况下的超声应力脉冲的表达式及其理论曲线,并给出了自由表面下的实验结果,都表明表面束缚时应力脉冲是单极性的,自由时是双极性的,应力脉冲增宽不大,其特性还受激光脉冲形状的影响.     

啁啾对飞秒脉冲在光子晶体光纤中传输的影响

采用广义非线性薛定谔方程描述啁啾对飞秒脉冲在光子晶体光纤中传输特性的影响,利用对称分步傅里叶方法通过求解方程,数值计算了有无啁啾情况下相同脉宽和功率、不同入射波长飞秒脉冲在光子晶体光纤中的传输,对比不同色散区飞秒脉冲波形的演化及超连续谱的产生.结果表明,较低功率时,反常色散区和零色散区,初始啁啾对于孤子的快速形成和传输具有重要的作用,而位于正常色散区时,啁啾破坏了脉冲形状,不利于脉冲的传输.反常色散区和正常色散区啁啾有利于频谱的展宽;零色散区,啁啾对频谱展宽影响不明显.较高功率时,频谱展宽主要受功率影响,啁啾对频谱展宽作用不大.这些结论对于脉冲传输和超连续谱系统优化设计和控制具有理论指导意义.     

用于测距的掺镱脉冲光纤激光器的输出特性

研究了用于测距的被动调Q掺镱光纤脉冲激光器的输出特性,仿真对比了可饱和吸收体长度以及增益光纤长度对输出功率的影响.结果表明:在抽运源功率为5 W的条件下,输出脉冲宽度为0.8μs,脉冲峰值功率为26 W,平均功率为2 W,脉冲能量为20μJ.在物体反射率为10%,探测距离为200 m,以及大气透过率为100%的条件下,返回最小功率为3.9×10~(-7) W.     

强子物质中重子离解XcJ截面的研究(英文)

在组分夸克交换模型中，从Buchmueller-Tye势出发得到夸克－夸克间的作用势，并应用这个作用势计算了强子物质中重子离解xcJ的截面，给出了主要反应道的截面对重子和粲偶素质心系能量的依赖。     

激光等离子体诱导Fe（CO）5解离制备超微铁粉

用ＴＥＡ－ＣＯ２脉冲激光器诱发反应介质击穿产生等离子体，导致Ｆｅ（ＣＯ）５气相解离获得超微纯铁粉，检测表明，超微粉粒径的１４０Ａ，质量很好，讨论了这一等离子体化学反应的特殊机理。     

用伪谱方法计算强激光场中一维原子的高次谐波和电离几率

引入非线性空间变换,用伪谱方法求解了一维原子在强激光场中的薛定谔方程,计算了一维原子在强激光场中的高次谐波和电离几率,其结果与分裂算符法得到的结果符合得很好.