| 新型材料固定化氧化还原酶进展 |
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| 引用本文： | 王世珍,刘凯泷,王世燕,江亮,段凌暄,熊雨,季哲惠.新型材料固定化氧化还原酶进展[J].福州大学学报(自然科学版),2021,49(4):568-576. |
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| 作者姓名： | 王世珍 刘凯泷 王世燕 江亮 段凌暄 熊雨 季哲惠 |
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| 作者单位： | 厦门大学化学化工学院化工系,厦门大学化学化工学院,厦门大学化学化工学院,厦门大学化学化工学院,厦门大学化学化工学院,厦门大学化学化工学院,厦门大学化学化工学院 |
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| 基金项目： | 国家自然科学基金项目（面上项目，重点项目，重大项目）,福建省自然科学基金资助项目（面上项目，重点项目，重大项目） |
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| 摘 要： | 氧化还原酶可催化许多关键反应，在生物制造中具有重要的应用价值。本文关注新型材料在氧化还原酶固定化中的应用和进展，总结碳材料、导电高分子、金属-有机框架材料等以及复合材料固定化酶的研究现状。分析各种材料的介观结构、理化性能，及其在酶固定中的优势和缺点。探讨以提高材料生物相容性从而提升氧化还原酶稳定性和催化效率为导向的界面修饰调控的策略。着重介绍导电材料固定化氧化还原酶，及其在生物转化、生物传感器、生物燃料电池等领域应用。并对氧化还原酶固定化的发展趋势和所面临的挑战进行展望。
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| 关 键 词： | 氧化还原酶 导电材料 生物电催化 生物电极 碳复合材料 金属-有机框架 |
| 收稿时间： | 2021/1/12 0:00:00 |
| 修稿时间： | 2021/3/3 0:00:00 |
Advance of new materials for the immobilization of oxidoreductases |
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| Wang Shizhen,Liu Kailong,Wang Shiyan,Jiang Liang,Duan Lingxuan,Xiong Yu and Ji Zhehui.Advance of new materials for the immobilization of oxidoreductases[J].Journal of Fuzhou University(Natural Science Edition),2021,49(4):568-576. |
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| Authors: | Wang Shizhen Liu Kailong Wang Shiyan Jiang Liang Duan Lingxuan Xiong Yu and Ji Zhehui |
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| Institution: | College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University,College of Chemistry and Chemical Engineering, Xiamen University |
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| Abstract: | Oxidoreductases catalyze a myriad of important reactions in biomanufacturing. Currently, various novel materials for oxidoreductases immobilization have been developed. Recent research based on carbon materials, conductive polymer, metal organic framework, and hybrids materials were reviewed. Chemical and physical characteristics of carriers with advantages and disadvantages were summarized. Strategies to improve the biocompatibility of carrier by surface modification and promote activity and stability of enzyme were addressed. Conductive materials for oxidoreductases immobilization and their application in bioelectrocatalysis, biosensor, and biofuel cells were discussed. Furthermore, challenges and perspectives in oxidoreductases immobilization are highlighted. |
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| Keywords: | oxidoreductases conductive materials bioelectrocatalysis biosensor hybrid carbon materials metal-organic framework |
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