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云水酸化数值模式计算探讨
引用本文:莫天麟,范靖.云水酸化数值模式计算探讨[J].南京大学学报(自然科学版),1987(3).
作者姓名:莫天麟  范靖
作者单位:南京大学大气科学系,南京大学大气科学系
摘    要:假定形成在硫酸盐和硝酸盐等核上的云滴溶解了酸、碱性气体,在很短时间内达到气液平衡,本文在先前的数值模式计算基础上,考虑大气中H_2O_2和O_3对SO_2的氧化过程对云水酸化的作用,并考虑云内液态含水量的改变对云水酸度的影响。计算结果表明:大气中SO_2的氧化过程对云水酸化的作用是不能忽视的,H_2O_2是一种比O_3更有效的氧化剂,而云中液态含水量改变对云水酸化的贡献相对地较小。

关 键 词:酸化  氧化剂  二氧化硫氧化  液态含水量  可溶性气体  气溶胶  模式计算

A STUDY OF THE CALCULATION OF NUMERICAL MODEL OF ACIDIFICATION OF CLOUD WATER
Mo Tianlin Fan Jing.A STUDY OF THE CALCULATION OF NUMERICAL MODEL OF ACIDIFICATION OF CLOUD WATER[J].Journal of Nanjing University: Nat Sci Ed,1987(3).
Authors:Mo Tianlin Fan Jing
Institution:Mo Tianlin Fan Jing
Abstract:It is assumed that the cloud droplets formed on sulfate and nitrate and other nuclei dissolve acidic and alkaline gases to achieve gas-liquid equilibrium in a very short time. In this paper, the considerations that oxidative process of SO_2 by H_2O_2 and O_3 in the atmosphere contributes to acidification of cloud water and that the change of liquid water content in cloud effects on acidity of cloud water are based on precedent the calculation of numerical model of acidification of cloud water. The result from calculations shows that the oxidative process of SO_2 in the atmosphere can not be negligible for the acidification of cloud water, that H_2O_2 is an oxidant stronger than O_3, and that the change of the liquid water content in cloud contributes relatively less to the acidification of cloud water.
Keywords:Acidification  Oxidant  SO_2 oxidation  Liquid water content  Soluble gases  aerosol  model calculation
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