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Nonlinear optical properties of Eu2O3 doped 5ZnO-20Nb2O5-75TeO2 glasses
Authors:Zhenyu?Zhao,Jiatian?Shi,Zhenrong?Sun  mailto:zrsun@phy.ecnu.edu.cn"   title="  zrsun@phy.ecnu.edu.cn"   itemprop="  email"   data-track="  click"   data-track-action="  Email author"   data-track-label="  "  >Email author,Jian?Lin,Wenhai?Huang,Zugeng?Wang
Affiliation:ZHAO Zhenyu1, SHI Jiatian1,2, SUN Zhenrong1, LIN Jian3, HUANG Wenhai3 & WANG Zugeng1 1. Key Laboratory of Optical and Magnetic Resonance Spectroscopy of the Ministry of Education, and Department of Physics, East China Normal University, Shanghai 200062, China; 2. Department of Physics, Nanning Teaching College, Nanning 530001, China; 3. School of Material Science and Engineering, Tongji University, Shanghai 200092, China Correspondence should be addressed to Sun Zhenrong
Abstract:
The third-order optical nonlinearities, including third-order nonlinear susceptibility c(3), nonlinear refractive index ( n2) and temporal response, were measured with forward DFWM using Nd:YAG mode-locked pulse laser. The results show that Eu2O3 doped 5ZnO-20Nb2O5-75TeO2 glasses have large n2 and ultra-fast temporal response. Raman spectra show that Eu2O3 dopant induces the changes in the local structure of glasses. The higher the dopant concentration, the larger the nonlinear refractive n2 and the faster the temporal response. The enhancement on the third-order optical nonlinearities can be attributed to the deformation of the electronic clouds in [TeO4] enhanced by Eu2O3 dopant.
Keywords:optical materials   Eu2O3 dopant   tellurite glass   DFWM   third-order optical nonlinear susceptibility.
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