Energy consumption of electrooxidation systems with boron-doped diamond electrodes in the pulse current mode |
| |
| Authors: | Jun-jun Wei Xu-hui Gao Li-fu Hei Jawaid Askari Cheng-ming Li |
| |
| Affiliation: | 1. Institute of Advanced Materials and Technology, University of Science and Technology Beijing, Beijing, 100083, China
2. Institute of Manufacturing Engineering, National University of Sciences & Technology (NUST), Habib Ibrahim Rehamat ullah Road, Karachi, 75350, Pakistan
|
| |
| Abstract: | A pulse current technique was conducted in a boron-doped diamond (BDD) anode system for electrochemical wastewater treatment. Due to the strong generation and weak absorption of hydroxyl radicals on the diamond surface, the BDD electrode possesses a powerful capability of electrochemical oxidation of organic compounds, especially in the pulse current mode. The influences of pulse current parameters such as current density, pulse duty cycle, and frequency were investigated in terms of chemical oxygen demand (COD) removal, average current efficiency, and specific energy consumption. The results demonstrated that the relatively high COD removal and low specific energy consumption were obtained simultaneously only if the current density or pulse duty cycle was adjusted to a reasonable value. Increasing the frequency slightly enhanced the COD removal and average current efficiency. A pulse-BDD anode system showed a stronger energy saving ability than a constant-BDD anode system when the electrochemical oxidation of phenol of the two systems was compared. The results prove that the pulse current technique is more cost-effective and more suitable for a BDD anode system for real wastewater treatment. A kinetic analysis was presented to explain the above results. |
| |
| Keywords: | |
| 本文献已被 万方数据 SpringerLink 等数据库收录！ |
| 点击此处可从《矿物冶金与材料学报》浏览原始摘要信息 |
|
点击此处可从《矿物冶金与材料学报》下载全文 |
|
